I think you'd have to bring the pressure down enough so that you boiled the water out of the balsa (without crushing it), or use vacuum + heat, or figure out a way to pull a vacuum but get airflow. None of these seem to be easy to me, although the vacuum + heat method might be doable with little more than the right bag material and a day in the kitchen when SWMBO isn't home.
If you could pull a vacuum and heat it up to 200 degrees F or whatever "wood bending" temperature is, you should get a better "mold", too.
At 20 degrees C (roughly room temperature) the vapor pressure of water is around 2.3kPa -- compare that to atmospheric pressure of about 100kPa. So at room temperature, to boil off the water in the balsa, you'd need to pull well over 29 inches. Even then, you'd only be just starting to make things boil, and who knows what water's affinity for wood does to the boiling point? You may end up squeezing more water out of the poor wood than you do boiling it off.
Bake things at 100C, and the vapor pressure of the water goes up to atmospheric -- so to get the stuff to boil off, you only need to pull a nominal vacuum. This means either:
- you can pull whatever you want to get the molding to work, or
- you'll dry that sucker out so bad it'll turn to dust when you let it cool.
Unfortunately, it looks like you have to get pretty close to 100C to start seeing real effects, because the vapor pressure is a mostly exponential function of temperature. See:
http://en.wikipedia.org/wiki/Vapour_pressure_of_water